Modeling and Optimization of Polymer based Bulk Heterojunction (BH) Solar cell

Abstract

A polymer phase separation model based on Cahn-Hilliard equation and a three-dimensional (3D) coupled exciton/electron/hole transport model in the disordered, phase-segregated morphology so generated, allow us to predict– possibly for the first time – the morphology dependent performance limits of polymer/fullerene bulk heterostructure (BH) solar cells. We relate the optimum anneal time to polymer sizes, solvent content, film thickness, and anneal temperature and find that a regularization of the morphology can double the efficiency of BH cells.

Keywords

Organic solar cell, Bulk Heterojunction, Process Model, Phase separation

Date of this Version

12-9-2009

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