Interfacial dynamics of drop coalescence and impinging liquid jets: Effect of viscous, Marangoni and shear-thinning stresses

Jiakai Lu, Purdue University

Abstract

The free-surface dynamics of drop coalescence and that of impinging liquid jets have both fundamental interest and practical importance in processes ranging from crop spraying and the processing of food emulsions to the atomization of fuel and propellants in combustion and propulsion engines. These processes frequently involve the use of complex fluids — shear-thinning or viscoelastic non-Newtonian liquids, which often contain surfactants either as additives or as contaminants. This thesis reports high-fidelity simulations of unsteady free-surface flows of complex fluids. The objective is to advance the understanding of the free-surface dynamics of drop coalescence and liquid jet impingement when viscous, surfactant and shear-thinning effects are important. Simulations in this thesis enabled, for the first time, a comprehensive numerical analysis of the coalescence of surfactant-laden drops after the merging drops make contact. The analysis reveals how interfacial (Marangoni) stresses induced by uneven accumulation of surfactant control the rate at which the drops coalesce by modulating the pull of surface tension on the tiny meniscus bridge joining the drops. Simulations also enabled the analysis of the unsteady free-surface dynamics of impinging viscous and shear-thinning liquid jets. Results demonstrate that viscous and shear-thinning stresses profoundly affects the impingement dynamics — in particular the velocity and thickness of the resulting radially expanding liquid sheet — by modifying the pressure developed in the impact region.

Degree

Ph.D.

Advisors

Sojka, Purdue University.

Subject Area

Mechanical engineering

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